Institut Charles Sadron Membre

Journal articles

titre

Triarylamine Trisamide Interfacial Modulation for Perovskite Photovoltaics

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Masaud Almalki, Ghewa Alsabeh, Marco A Ruiz‐preciado, Hong Zhang, Melodie Galerne, Emilie Moulin, Felix Thomas Eickemeyer, Shaik M Zakeeruddin, Jovana V Milić, Nicolas Giuseppone, Michael Grätzel

article

Advanced Materials Interfaces, 2024, pp.2301053. ⟨10.1002/admi.202301053⟩

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Hybrid perovskites stand out as one of the leading materials in the new generation of photovoltaics. .....

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DOI : 10.1002/admi.202301053

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Molecular actuation of a bistable liquid-crystalline [c2]daisy chain rotaxane

auteur

Christian C Carmona-Vargas, Lara Faour, Shoichi Tokunaga, Doru Constantin, Guillaume Fleith, Emilie Moulin, Nicolas Giuseppone

article

ChemistryEurope, 2024, 2 (1), pp.e202300069. ⟨10.1002/ceur.202300069⟩

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A bistable [c2]daisy chain rotaxane bearing two mesogen units was synthesized, and its liquid crysta .....

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DOI : 10.1002/ceur.202300069

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Out‐of‐Equilibrium Mechanical Disruption of β‐Amyloid‐Like Fibers using Light‐Driven Molecular Motors

auteur

Dania Daou, Yohan Zarate, Mounir Maaloum, Dominique Collin, Guillaume Fleith, Doru Constantin, Emilie Moulin, Nicolas Giuseppone

article

Advanced Materials, 2024, 36 (18), pp.2311293. ⟨10.1002/adma.202311293⟩

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Artificial molecular motors have the potential to generate mechanical work on their environment by p .....

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DOI : 10.1002/adma.202311293

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Thermodynamics, morphology and molecular structure of molecular compounds in trisamide triarylamine organogels and pseudo-organogels

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Ganesh Viswanatha-Pillai, Andreas Vargas-Jentzsch, Alain Carvalho, Guillaume Fleith, Odile Gavat, Emilie Moulin, Nicolas Giuseppone, Jean-Michel Guenet

article

Soft Matter, 2023, 19 (25), pp.4660-4668. ⟨10.1039/d3sm00624g⟩

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In this paper, potentially-gelling binary systems are investigated by DSC, X-ray and Electron micros .....

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DOI : 10.1039/d3sm00624g

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Bending Actuation of Hydrogels through Rotation of Light‐Driven Molecular Motors

auteur

Alexis Perrot, Wen‐zhi Wang, Eric Buhler, Emilie Moulin, Nicolas Giuseppone

article

Angewandte Chemie International Edition, 2023, ⟨10.1002/anie.202300263⟩

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DOI : 10.1002/anie.202300263

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Daisy chain architectures: from discrete molecular entities to polymer materials

auteur

Emilie Moulin, Christian C Carmona-Vargas, Nicolas Giuseppone

article

Chemical Society Reviews, 2023, 52 (21), pp.7333-7358. ⟨10.1039/d3cs00619k⟩

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We review recent progresses in the synthesis and the use of daisy chain architectures as molecular m .....

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DOI : 10.1039/d3cs00619k

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Evidence by neutron diffraction of molecular compounds in triarylamine tris-amide organogels and in their hybrid thermoreversible gels with PVC

auteur

J.-M. Guenet, B. Demé, O. Gavat, E. Moulin, N. Giuseppone

article

Soft Matter, 2022, 18 (14), pp.2851-2857. ⟨10.1039/d2sm00254j⟩

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We report on neutron diffraction experiments performed on organogels prepared from triarylamine tris .....

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DOI : 10.1039/d2sm00254j

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Effect of solvent isomers on the gelation properties of tri-aryl amine organogels and their hybrid thermoreversible gels with poly[vinyl chloride]

auteur

Xiao Yao, Dominique Collin, Odile Gavat, Alain Carvalho, Moulin Emilie, Nicolas Giuseppone, Jean-Michel Guenet

article

Soft Matter, 2022, 18 (30), pp.5575 - 5584. ⟨10.1039/d2sm00563h⟩

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The gelation properties of tri-aryl amine (TATA) in two isomers of dichlorobenzene, namely orthodich .....

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DOI : 10.1039/d2sm00563h

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titre

Some Remarkable Rheological and Conducting Properties of Hybrid PVC Thermoreversible Gels/Organogels

auteur

Dominique Collin, Ganesh Viswanatha-Pillai, Andreas Vargas Jentzsch, Odile Gavat, Emilie Moulin, Nicolas Giuseppone, Jean-Michel Guenet

article

Gels, 2022, 8 (9), pp.557. ⟨10.3390/gels8090557⟩

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We report on investigations into the rheological properties of organogels prepared from triarylamine .....

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DOI : 10.3390/gels8090557

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titre

Light-Driven Molecular Whirligig

auteur

Chuan Gao, Andreas Vargas Jentzsch, Emilie Moulin, Nicolas Giuseppone

article

Journal of the American Chemical Society, 2022, 144 (22), pp.9845-9852. ⟨10.1021/jacs.2c02547⟩

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An unidirectional light-driven rotary motor was looped in a figure-of-eight molecule by linking two .....

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DOI : 10.1021/jacs.2c02547

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Journal articles

titre

Extraction of mechanical work from stimuli-responsive molecular systems and materials

auteur

Alexis Perrot, Emilie Moulin, Nicolas Giuseppone

article

Trends in Chemistry, 2021, 3 (11), pp.926-942. ⟨10.1016/j.trechm.2021.08.007⟩

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Molecular switches and advanced molecular motors, which are the elementary building blocks for the c .....

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DOI : 10.1016/j.trechm.2021.08.007

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Design of Stimuli-Responsive Dynamic Covalent Delivery Systems for Volatile Compounds (Part 2): Fragrance-Releasing Cleavable Surfactants in Functional Perfumery Applications

auteur

Vera Tchakalova, Eric Lutz, Serge Lamboley, Emilie Moulin, Daniel Benczédi, Nicolas Giuseppone, Andreas Herrmann

article

Chemistry - A European Journal, 2021, 27 (53), pp.13468-13476. ⟨10.1002/chem.202102051⟩

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Amphiphilic imines prepared by condensation of a hydrophobic fragrance aldehyde with a hydrophilic a .....

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DOI : 10.1002/chem.202102051

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Modulation of the Molecular Structure of Tri-aryl Amine Fibrils in Hybrid Poly[vinyl chloride] Gel/Organogel Systems

auteur

Parniyan Talebpour, Benoît Heinrich, Odile Gavat, Alain Carvalho, Emilie Moulin, Nicolas Giuseppone, Jean-Michel Guenet

article

Macromolecules, 2021, 54 (17), pp.8104-8111. ⟨10.1021/acs.macromol.1c01282⟩

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This paper reports on the thermodynamics through mapping out temperature−concentration phase diagr .....

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DOI : 10.1021/acs.macromol.1c01282

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Supramolecular Polymerization of Triarylamine-Based Macrocycles into Electroactive Nanotubes

auteur

Flavio Picini, Susanne Schneider, Odile Gavat, Andreas Vargas Jentzsch, Junjun Tan, Mounir Maaloum, Jean-Marc Strub, Shoichi Tokunaga, Jean-Marie Lehn, Emilie Moulin, Nicolas Giuseppone

article

Journal of the American Chemical Society, 2021, 143 (17), pp.6498-6504. ⟨10.1021/jacs.1c00623⟩

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A S6-symmetric triarylamine-based macrocycle (i.e. hexaaza[16]para-cyclophane), decorated with six l .....

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DOI : 10.1021/jacs.1c00623

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Light-Driven Molecular Motors Boost the Selective Transport of Alkali Metal Ions through Phospholipid Bilayers

auteur

Wen-Zhi Wang, Li-Bo Huang, Shao-Ping Zheng, Emilie Moulin, Odile Gavat, Mihail Barboiu, Nicolas Giuseppone

article

Journal of the American Chemical Society, 2021, 143 (38), pp.15653-15660. ⟨10.1021/jacs.1c05750⟩

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A hydrophobic light-driven rotary motor is functionalized with two 18-crown-6 macrocycles and incorp .....

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DOI

DOI : 10.1021/jacs.1c05750

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titre

Design of Stimuli-Responsive Dynamic Covalent Delivery Systems for Volatile Compounds (Part 1): Controlled Hydrolysis of Micellar Amphiphilic Imines in Water

auteur

Eric Lutz, Emilie Moulin, Vera Tchakalova, Daniel Benczédi, Andreas Herrmann, Nicolas Giuseppone

article

Chemistry - A European Journal, 2021, 27 (53), pp.13457-13467. ⟨10.1002/chem.202102049⟩

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Despite their intrinsic hydrolysable character, imine bonds can become remarkably stable in water wh .....

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DOI : 10.1002/chem.202102049

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Journal articles

titre

Hybrid materials from tri-aryl amine organogelators and poly[vinyl chloride] networks

auteur

Bethelihim Kiflemariam, Dominique Collin, Odile Gavat, Alain Carvalho, Emilie Moulin, Nicolas Giuseppone, Jean-Michel Guenet

article

Polymer, 2020, 207, pp.122814. ⟨10.1016/j.polymer.2020.122814⟩

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Hybrid thermoreversible gels have been prepared from polyvinyl chloride (PVC) and tri-aryl tri-amine .....

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DOI : 10.1016/j.polymer.2020.122814

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titre

From Molecular Machines to Stimuli‐Responsive Materials

auteur

Emilie Moulin, Lara Faour, Christian Carmona‐vargas, Nicolas Giuseppone

article

Advanced Materials, 2020, 32 (20), pp.1906036. ⟨10.1002/adma.201906036⟩

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DOI : 10.1002/adma.201906036

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titre

Design of Collective Motions from Synthetic Molecular Switches, Rotors, and Motors

auteur

Damien Dattler, Gad Fuks, Joakim Heiser, Emilie Moulin, Alexis Perrot, Xuyang Yao, Nicolas Giuseppone

article

Chemical Reviews, 2020, 120 (1), pp.310-433. ⟨10.1021/acs.chemrev.9b00288⟩

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Precise control over molecular movement is of fundamental and practical importance in physics, biolo .....

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DOI : 10.1021/acs.chemrev.9b00288

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Structural properties of contractile gels based on light-driven molecular motors: a small-angle neutron and X-ray study

auteur

Giacomo Mariani, Jean-Rémy Colard-Itté, Emilie Moulin, Nicolas Giuseppone, Eric Buhler

article

Soft Matter, 2020, 16 (16), pp.4008-4023. ⟨10.1039/d0sm00031k⟩

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The detailed structure of active polymer gels built by integrating light-driven rotary molecular mot .....

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DOI : 10.1039/d0sm00031k

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Homodyne dynamic light scattering in supramolecular polymer solutions: anomalous oscillations in intensity correlation function

auteur

Emilie Moulin, Irina Nyrkova, Nicolas Giuseppone, Alexander Semenov, Eric Buhler

article

Soft Matter, 2020, 16 (12), pp.2971-2993. ⟨10.1039/c9sm02480h⟩

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Dilute solutions of electronically active molecules capable of irradiation-driven supramolecular sel .....

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DOI : 10.1039/c9sm02480h

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Journal articles

titre

Covalently Trapped Triarylamine‐Based Supramolecular Polymers

auteur

Ting Liang, Dominique Collin, Melodie Galerne, Gad Fuks, Andreas Vargas Jentzsch, Mounir Maaloum, Alain Carvalho, Nicolas Giuseppone, Emilie Moulin

article

Chemistry - A European Journal, 2019, 25 (63), pp.14341-14348. ⟨10.1002/chem.201902404⟩

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DOI : 10.1002/chem.201902404

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titre

Temperature Control of Sequential Nucleation–Growth Mechanisms in Hierarchical Supramolecular Polymers

auteur

Artem Osypenko, Emilie Moulin, Odile Gavat, Gad Fuks, Mounir Maaloum, Mark Koenis, Wybren Jan Buma, Nicolas Giuseppone

article

Chemistry - A European Journal, 2019, 25 (56), pp.13008-13016. ⟨10.1002/chem.201902898⟩

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Upon cooling in solution, chiral triarylamine tris-amide unimers produce organogels by stacking into .....

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DOI : 10.1002/chem.201902898

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Unsymmetric bistable [c2]daisy chain rotaxanes which combine two types of electroactive stoppers

auteur

Adrian Wolf, Juan-José Cid, Emilie Moulin, Frédéric Niess, Guangyan Du, Antoine Goujon, Eric Busseron, Adrian Ruff, Sabine Ludwigs, Nicolas Giuseppone

article

European Journal of Organic Chemistry, 2019, 2019 (21), pp.3421-3432. ⟨10.1002/ejoc.201900179⟩

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Mechanically interlocked molecules (MIMs) have emerged as intriguing building blocks for the constru .....

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DOI : 10.1002/ejoc.201900179

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Triarylamine-Based Supramolecular Polymers: Structures, Dynamics, and Functions

auteur

Emilie Moulin, Joseph J Armao, Nicolas Giuseppone

article

Accounts of Chemical Research, 2019, 52 (4), pp.975-983. ⟨10.1021/acs.accounts.8b00536⟩

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Triarylamine molecules and triarylamine-based covalent polymers have been extensively investigated f .....

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DOI : 10.1021/acs.accounts.8b00536

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Mechanical behaviour of contractile gels based on light-driven molecular motors

auteur

Jean-Rémy Colard-Itté, Quan Li, Dominique Collin, Giacomo Mariani, Gad Fuks, Emilie Moulin, Eric Buhler, Nicolas Giuseppone

article

Nanoscale, 2019, 11 (12), pp.5197-5202. ⟨10.1039/C9NR00950G⟩

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The networking of individual artificial molecular motors into collective actuation systems is a prom .....

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DOI : 10.1039/C9NR00950G

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Journal articles

titre

Supramolecular Electropolymerization

auteur

Thomas Ellis, Melodie Galerne, Joseph Armao, Artem Osypenko, David Martel, Mounir Maaloum, Gad Fuks, Odile Gavat, Emilie Moulin, Nicolas Giuseppone

article

Angewandte Chemie International Edition, 2018, 57 (48), pp.15749-15753. ⟨10.1002/anie.201809756⟩

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Gaining control over supramolecular polymerization mechanisms is of high fundamental interest to und .....

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DOI : 10.1002/anie.201809756

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3D supramolecular self-assembly of [60]fullerene hexaadducts decorated with triarylamine molecules

auteur

Odile Gavat, Thi Minh Nguyet Trinh, Emilie Moulin, Thomas Ellis, Mounir Maaloum, Eric Buhler, Guillaume Fleith, Jean-François Nierengarten, Nicolas Giuseppone

article

Chemical Communications, 2018, 54 (55), pp.7657-7660. ⟨10.1039/C8CC04079F⟩

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DOI : 10.1039/C8CC04079F

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titre

Dual-light control of nanomachines that integrate motor and modulator subunits

auteur

Justin Foy, Quan Li, Antoine Goujon, Jean-Rémy Colard-Itté, Gad Fuks, Emilie Moulin, Olivier Schiffmann, Damien Dattler, Daniel Funeriu, Nicolas Giuseppone

article

Nature Nanotechnology, 2017, 12 (6), pp.540-545. ⟨10.1038/nnano.2017.28⟩

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DOI : 10.1038/nnano.2017.28

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titre

Columnar Self-Assemblies of Triarylamines as Scaffolds for Artificial Biomimetic Channels for Ion and for Water Transport

auteur

Susanne Schneider, Erol-Dan Licsandru, Istvan Kocsis, Arnaud Gilles, Florina Dumitru, Emilie Moulin, Junjun Tan, Jean-Marie Lehn, Nicolas Giuseppone, Mihail Barboiu

article

Journal of the American Chemical Society, 2017, 139 (10), pp.3721 - 3727. ⟨10.1021/jacs.6b12094⟩

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DOI : 10.1021/jacs.6b12094

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Anisotropic Self-Assembly of Supramolecular Polymers and Plasmonic Nanoparticles at the Liquid–Liquid Interface

auteur

Joseph Armao, Irina Nyrkova, Gad Fuks, Artem Osypenko, Mounir Maaloum, Emilie Moulin, Raul Arenal, Odile Gavat, Alexander Semenov, Nicolas Giuseppone

article

Journal of the American Chemical Society, 2017, 139 (6), pp.2345-2350. ⟨10.1021/jacs.6b11179⟩

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The study of supramolecular polymers in the bulk, in diluted solution, and at the solid-liquid inter .....

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DOI : 10.1021/jacs.6b11179

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Integration of molecular machines into supramolecular materials: actuation between equilibrium polymers and crystal-like gels

auteur

Giacomo Mariani, Antoine Goujon, Emilie Moulin, Michel Rawiso, Nicolas Giuseppone, Eric Buhler

article

Nanoscale, 2017, 9 (46), pp.18456-18466. ⟨10.1039/C7NR04251E⟩

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In this article, the dynamic structure of complex supramolecular polymers composed of bistable [c2]d .....

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DOI : 10.1039/C7NR04251E

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Bistable [ c 2] Daisy Chain Rotaxanes as Reversible Muscle-like Actuators in Mechanically Active Gels

auteur

Antoine Goujon, Thomas Lang, Giacomo Mariani, Emilie Moulin, Gad Fuks, Jesus Raya, Eric Buhler, Nicolas Giuseppone

article

Journal of the American Chemical Society, 2017, 139 (42), pp.14825-14828. ⟨10.1021/jacs.7b06710⟩

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The implementation of molecular machines in polymer science is of high interest to transfer mechanic .....

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DOI : 10.1021/jacs.7b06710

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Controlled Sol–Gel Transitions by Actuating Molecular Machine Based Supramolecular Polymers

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Antoine Goujon, Giacomo Mariani, Thomas Lang, Emilie Moulin, Michel Rawiso, Eric Buhler, Nicolas Giuseppone

article

Journal of the American Chemical Society, 2017, 139 (13), pp.4923-4928. ⟨10.1021/jacs.7b00983⟩

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The implementation of artificial molecular machines in polymer science is an important objective tha .....

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DOI : 10.1021/jacs.7b00983

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Supramolecular Organic Nanowires as Plasmonic Interconnects

auteur

Joseph Armao, Yuya Domoto, Teruhiko Umehara, Mounir Maaloum, Christophe Contal, Gad Fuks, Emilie Moulin, Gero Decher, Nicolas Javahiraly, Nicolas Giuseppone

article

ACS Nano, 2016, 10 (2), pp.2082-2090. ⟨10.1021/acsnano.5b06294⟩

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DOI : 10.1021/acsnano.5b06294

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Self-assembly of supramolecular triarylamine nanowires in mesoporous silica and biocompatible electrodes thereof

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Erol-Dan Licsandru, Susanne Schneider, Sophie Tingry, Thomas Ellis, Emilie Moulin, Mounir Maaloum, Jean-Marie Lehn, Mihail Barboiu, Nicolas Giuseppone

article

Nanoscale, 2016, 8 (10), pp.5605 - 5611. ⟨10.1039/c5nr06977g⟩

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Biocompatible silica-based mesoporous materials, which present high surface areas combined with unif .....

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DOI : 10.1039/c5nr06977g

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Hydrogen-Bonded Multifunctional Supramolecular Copolymers in Water

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Yunjie Xiang, Emilie Moulin, Eric Buhler, Mounir Maaloum, Gad Fuks, Nicolas Giuseppone

article

Langmuir, 2015, 31 (28), pp.7738-7748. ⟨10.1021/acs.langmuir.5b01093⟩

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We have investigated the self-assembly in water of molecules having a single hydrophobic bis-urea do .....

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DOI : 10.1021/acs.langmuir.5b01093

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Light-Controlled Morphologies of Self-Assembled Triarylamine–Fullerene Conjugates

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Eric Busseron, Juan-José Cid, Adrian Wolf, Guangyan Du, Emilie Moulin, Gad Fuks, Mounir Maaloum, Prasad Polavarapu, Adrian Ruff, Ann-Kathrin Saur, Sabine Ludwigs, Nicolas Giuseppone

article

ACS Nano, 2015, 9 (3), pp.2760-2772. ⟨10.1021/nn506646m⟩

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A family of triarylamine–fullerene conjugates has been synthesized and shown to self-assemble upon .....

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DOI : 10.1021/nn506646m

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Macroscopic contraction of a gel induced by the integrated motion of light-driven molecular motors

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Quan Li, Gad Fuks, Emilie Moulin, Mounir Maaloum, Michel Rawiso, Igor Kulic, Justin Foy, Nicolas Giuseppone

article

Nature Nanotechnology, 2015, 10 (2), pp.161-165. ⟨10.1038/nnano.2014.315⟩

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DOI : 10.1038/nnano.2014.315

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pH and light-controlled self-assembly of bistable [c2] daisy chain rotaxanes

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Adrian Wolf, Emilie Moulin, Juan Jose Cid Martin, Antoine Goujon, Guangyan Du, Eric Busseron, Gad Fuks, Nicolas Giuseppone

article

Chemical Communications, 2015, 51 (20), pp.4212-4215. ⟨10.1039/C4CC10331A⟩

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A logic gate based on a bistable [c2] daisy chain rotaxane decorated with lateral triarylamine units .....

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DOI : 10.1039/C4CC10331A

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Light Scattering Strategy for the Investigation of Time-Evolving Heterogeneous Supramolecular Self-Assemblies

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Nicolas Jouault, Emilie Moulin, Nicolas Giuseppone, Eric Buhler

article

Physical Review Letters, 2015, 115, ⟨10.1103/PhysRevLett.115.085501⟩

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Supramolecular self-assembly is a multiple length-scale and time-dependent process involving many co .....

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DOI : 10.1103/PhysRevLett.115.085501

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Supramolecular Self-Assembly and Radical Kinetics in Conducting Self-Replicating Nanowires

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Irina Nyrkova, Emilie Moulin, Joseph Armao, Mounir Maaloum, Benoit Heinrich, Michel Rawiso, Frederic Niess, Juan Jose Cid, Nicolas Jouault, Eric Buhler, Alexander Semenov, Nicolas Giuseppone

article

ACS Nano, 2014, 8 (10), pp.10111-10124. ⟨10.1021/nn502863b⟩

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By using a combination of experimental and theoretical tools, we elucidate unique physical character .....

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DOI : 10.1021/nn502863b

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A move in the right direction

auteur

Emilie Moulin, Nicolas Giuseppone

article

Nature Nanotechnology, 2014, 9 (5), pp.331-332. ⟨10.1038/nnano.2014.91⟩

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DOI : 10.1038/nnano.2014.91

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Experimental and theoretical methods for the analyses of dynamic combinatorial libraries

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Maria Cristina Misuraca, Emilie Moulin, Yves Ruff, Nicolas Giuseppone

article

New Journal of Chemistry, 2014, 38 (8), pp.3336-3349. ⟨10.1039/C4NJ00304G⟩

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Because of their recent interest towards dynamic combinatorial systems, chemists have to challenge t .....

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DOI : 10.1039/C4NJ00304G

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Muscle-like Supramolecular Polymers: Integrated Motion from Thousands of Molecular Machines

auteur

Guangyan Du, Emilie Moulin, Nicolas Jouault, Eric Buhler, Nicolas Giuseppone

article

Angewandte Chemie International Edition, 2012, 51 (50), pp.12504-12508. ⟨10.1002/anie.201206571⟩

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DOI : 10.1002/anie.201206571

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Light triggered self-construction of supramolecular organic nanowires as metallic interconnects

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Vina Faramarzi, Frédéric Niess, Emilie Moulin, Mounir Maaloum, Jean-François Dayen, Jean-Baptiste Beaufrand, Silvia Zanettini, Bernard Doudin, Nicolas Giuseppone

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Nature Chemistry, 2012, 4 (6), pp.485-490. ⟨10.1038/nchem.1332⟩

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The construction of soft and processable organic material able to display metallic conduction proper .....

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DOI : 10.1038/nchem.1332

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Hierarchical supramolecular structuring and dynamical properties of water soluble polyethylene glycol-perylene self-assemblies

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Nicolas Jouault, Yunjie Xiang, Emilie Moulin, Gad Fuks, Nicolas Giuseppone, Eric Buhler

article

Physical Chemistry Chemical Physics, 2012, 14 (16), pp.5718-5728. ⟨10.1039/c2cp23786e⟩

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DOI : 10.1039/c2cp23786e

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Light-triggered self-assembly of triarylamine-based nanospheres

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Emilie Moulin, Frédéric Niess, Gad Fuks, Nicolas Jouault, Eric Buhler, Nicolas Giuseppone

article

Nanoscale, 2012, 4 (21), pp.6748. ⟨10.1039/c2nr32168h⟩

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DOI : 10.1039/c2nr32168h

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The Hierarchical Self-Assembly of Charge Nanocarriers: A Highly Cooperative Process Promoted by Visible Light

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Emilie Moulin, Fréderic Niess, Mounir Maaloum, Eric Buhler, Irina Nyrkova, Nicolas Giuseppone

article

Angewandte Chemie International Edition, 2010, 49 (39), pp.6974-6978. ⟨10.1002/anie.201001833⟩

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Let there be more light: Triarylamine-based building blocks respond to visible-light exposure by the .....

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DOI

DOI : 10.1002/anie.201001833

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